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We search for dark matter in the form of axionlike particles (ALPs) in the mass range by probing their possible coupling to fermion spins through the ALP field gradient. This is achieved by performing proton nuclear magnetic resonance spectroscopy on a sample of methanol as a technical demonstration of the Cosmic Axion Spin Precession Experiment Gradient (CASPEr-Gradient) Low-Field apparatus. Searching for spin-coupled ALP dark matter in this mass range with associated Compton frequencies in a 240 Hz window centered at 1.348570 MHZ resulted in a sensitivity to the ALP-proton coupling constant of . This narrow-bandwidth search serves as a proof-of-principle and a commissioning measurement, validating our methodology and demonstrating the experiment’s capabilities. CASPEr-Gradient Low-Field will probe the mass range from to with hyperpolarized samples to boost the sensitivity beyond the astronomical limits.more » « lessFree, publicly-accessible full text available September 1, 2026
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Gkika, Violeta; Kim, Younggeun; Matlashov, Andrei; Shin, Yun Chang; Semertzidis, Yannis; Cantor, Robin; Lohmeyer, Chloe; Aggarwal, Nancy; Geraci, Andrew (, Journal of Low Temperature Physics)ARIADNE (Axion Resonant InterAction Detection Experiment) is a table-top experiment that intends to search for QCD axions from exotic spin-dependent interactions mediated by axion between nuclei at sub-mm range. This experiment includes a non-magnetic mass to source the axion field, and a dense ensemble of hyper-polarized 3He nuclei to detect the axion field with nuclear-magnetic-resonance (NMR)-based method. The expected NMR signal from the interaction could be easily buried in the noise spectrum of the magnetometer, especially in a frequency range (~ 100 Hz) where the interaction signal is supposed to exist. In this work, we report optimization of SQUID gradiometer for ARIADNE including noise spectrum measurement.more » « less
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Kim, Dongok; Kimball, Derek F.; Masia-Roig, Hector; Smiga, Joseph A.; Wickenbrock, Arne; Budker, Dmitry; Kim, Younggeun; Shin, Yun Chang; Semertzidis, Yannis K. (, Physics of the Dark Universe)
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